Published August 1, 2009 | Version public
Journal Article

Oxygen isotopic composition of chondritic interplanetary dust particles: A genetic link between carbonaceous chondrites and comets

  • 1. ROR icon Lawrence Livermore National Laboratory
  • 2. ROR icon Centre de Recherches Pétrographiques et Géochimiques
  • 3. ROR icon University of California, Los Angeles
  • 4. ROR icon Laboratoire de Physique des 2 Infinis Irène Joliot-Curie
  • 5. ROR icon Goddard Space Flight Center

Abstract

Oxygen isotopes were measured in four chondritic hydrated interplanetary dust particles (IDPs) and five chondritic anhydrous IDPs including two GEMS-rich particles (Glass embedded with metal and sulfides) by a combination of high precision and high lateral resolution ion microprobe techniques. All IDPs have isotopic compositions tightly clustered around that of solar system planetary materials. Hydrated IDPs have mass-fractionated oxygen isotopic compositions similar to those of CI and CM carbonaceous chondrites, consistent with hydration of initially anhydrous protosolar dust. Anhydrous IDPs have small 16O excesses and depletions similar to those of carbonaceous chondrites, the largest ¹⁶O variations being hosted by the two GEMS-rich IDPs. Coarse-grained forsteritic olivine and enstatite in anhydrous IDPs are isotopically similar to their counterparts in comet Wild 2 and in chondrules suggesting a high temperature inner solar system origin. The small variations in the ¹⁶O content of GEMS-rich IDPs suggest that most GEMS either do not preserve a record of interstellar processes or the initial interstellar dust is not ¹⁶O-rich as expected by self-shielding models, although a larger dataset is required to verify these conclusions. Together with other chemical and mineralogical indicators, O isotopes show that the parent-bodies of carbonaceous chondrites, of chondritic IDPs, of most Antarctic micrometeorites, and comet Wild 2 belong to a single family of objects of carbonaceous chondrite chemical affinity as distinct from ordinary, enstatite, K- and R-chondrites. Comparison with astronomical observations thus suggests a chemical continuum of objects including main belt and outer solar system asteroids such as C-type, P-type and D-type asteroids, Trojans and Centaurs as well as short-period comets and other Kuiper Belt Objects.

Additional Information

We would like to thank John Bradley and Don Brownlee for providing the IDPs studied in 1999 and the curation team at the Johnson Space Center for providing the IDPs studied in 2005. Ian Hutcheon is warmly thanked for hosting one of us (JA) during the 2005 session. Together with JEOL, he also provided necessary help with the brand new LLNL FEG-SEM. All the ion probe group in Nancy is warmly thanked for discussions, help and maintenance of the IMS 1270 during the 2003–2004 "small beam analysis" development sessions. Alice Aléon-Toppani is thanked for numerous discussions about the nature of GEMS. Advice from Rick Ryerson and Mike Toplis about oxygen self-diffusion is appreciated. We would like to thank in-depth revision and advices from the associate editor Christian Koeberl, from Matthew Genge and two other anonymous reviewers. The UCLA ion probe laboratory is partially supported by the NSF Instrumentation and Facilities program. This work was supported by a grant from the NASA Cosmochemistry program and by the LLNL Institute of Geophysics and Planetary Physics. This work was performed under the auspices of the US Department of Energy by the Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344.

Additional details

Identifiers

Eprint ID
119721
Resolver ID
CaltechAUTHORS:20230307-650012000.16

Funding

NASA
Lawrence Livermore National Laboratory
Department of Energy (DOE)
DE-AC52-07NA27344

Dates

Created
2023-03-12
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Updated
2023-03-12
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