Published March 1, 2015 | Version Published
Journal Article Open

A sensitivity analysis to assess the relative importance of improvements in electrocatalysts, light absorbers, and system geometry on the efficiency of solar-fuels generators

  • 1. ROR icon Joint Center for Artificial Photosynthesis
  • 2. ROR icon Division of Chemistry
  • 3. ROR icon California Institute of Technology

Abstract

A sensitivity analysis has been performed for a variety of generic designs for solar-fuels generators. The analysis has revealed the relative importance of reductions in the overpotentials of electrocatalysts, of improvements in the materials properties of light absorbers, and of optimization in the system geometry for various different types of solar-fuels generators, while considering operation at a range of temperatures as well as under a variety of illumination intensities including up to 10-fold optical concentration.

Additional Information

© 2015 The Royal Society of Chemistry. Received 23 Jul 2014, Accepted 23 Dec 2014, First published online 24 Dec 2014. This material is based upon work performed by the Joint Center for Artificial Photosynthesis, a DOE Energy Innovation Hub, supported through the Office of Science of the U.S. Department of Energy under Award number DE-SC0004993.

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Identifiers

Eprint ID
57103
Resolver ID
CaltechAUTHORS:20150430-084157336

Funding

Department of Energy (DOE)
DE-SC0004993

Dates

Created
2015-04-30
Created from EPrint's datestamp field
Updated
2021-11-10
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