CaltechAUTHORS
Published February 6, 2015 | Version Published
Journal Article Open

Competing reaction processes on a lattice as a paradigm for catalyst deactivation

Creators

  • 1. ROR icon University of Extremadura
  • 2. ROR icon DePaul University
  • 3. ROR icon California Institute of Technology

Abstract

We mobilize both a generating function approach and the theory of finite Markov processes to compute the probability of irreversible absorption of a randomly diffusing species on a lattice with competing reaction centers. We consider an N-site lattice populated by a single deep trap, and N−1 partially absorbing traps (absorption probability 0

Additional Information

© 2015 American Physical Society. Received 31 July 2014; published 6 February 2015. E.A. gratefully acknowledges financial support from the Spanish Government through Grant No. FIS2013-42840-P (partially funded by FEDER funds) as well as additional financial support from Junta de Extremadura through Grant No. GR10158. Part of this study was carried out while E.A. was a visiting professor at DePaul University, and while J.J.K. was in residence at the Beckman Institute. The latter author thanks H. B. Gray for his support and generous hospitality.

Attached Files

Published - PhysRevE.91.022106.pdf

Files

PhysRevE.91.022106.pdf

Files (223.3 kB)

Name Size
md5:bc8ff72d0f11975ff0a7c70db1a03a14
223.3 kB Preview Download

Additional details

Identifiers

Eprint ID
55631
Resolver ID
CaltechAUTHORS:20150309-095732008

Funding

Spanish Government
FIS2013-42840-P
FEDER Funds
Junta de Extremadura
GR10158

Dates

Created
2015-03-10
Created from EPrint's datestamp field
Updated
2021-11-10
Created from EPrint's last_modified field